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3 October 2022 Tunable nonlinear vibrational response of monolayer hBN
Fadil Iyikanat, Andrea Konecna, Javier García de Abajo
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Proceedings Volume PC12228, Ultrafast Nonlinear Imaging and Spectroscopy X; PC122280K (2022) https://doi.org/10.1117/12.2633142
Event: SPIE Optical Engineering + Applications, 2022, San Diego, California, United States
Abstract
Nonlinear optical processes resulting from the interaction of light with matter have provided great opportunities in photonics technologies by enabling spectral control of light. Here, based on first-principles calculations, we investigate the linear and nonlinear optical response of monolayer hBN in the mid-infrared polaritonic region following time-domain and perturbative schemes, from which we conclude an extraordinarily large nonlinear response, which can be modulated by lateral electrical gating and presents an opportunity to achieve quantum blockade at the level of a few quanta. Our study reveals a range of potential applications that include harmonic generation, optical modulation, and quantum information in the mid-infrared range.
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Fadil Iyikanat, Andrea Konecna, and Javier García de Abajo "Tunable nonlinear vibrational response of monolayer hBN", Proc. SPIE PC12228, Ultrafast Nonlinear Imaging and Spectroscopy X, PC122280K (3 October 2022); https://doi.org/10.1117/12.2633142
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KEYWORDS
Mid-IR
Modulation
Nonlinear response
Optoelectronics
Kerr effect
Nonlinear optics
Phonons
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