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Achieving condensed phase optical refrigeration requires near-unity emission quantum yields (QYs). Colloidal CsPbBr3 nanocrystals (NCs) are promising candidates in this respect given near unity QY-values, achieved by post-synthetic surface treatment with quaternary ammonium bromide ligands. The origin of these QY enhancements, however, is not understood. Systematic nuclear magnetic resonance studies of the organic ligand passivation of near unity QY CsPbBr3 NC surfaces are therefore conducted to better reveal their surface-ligand interactions.
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