Molecular ensembles in confined infrared (IR) fields have emerged as a promising platform for condensed-phase cavity QED at room temperature, for the development of scalable architectures for IR quantum optics also at the nanoscale. We develop a Markovian open quantum system approach to study the dynamics of molecular vibrations in infrared nanocavities under femtosecond pulse driving, as implemented in recent nanoprobe spectroscopy experiments with polymer-coated IR gold antennas. We describe the time-domain signatures of the crossover from weak to strong coupling regimes in these nanocavities, provide mechanistic insights on the conditions for implementing coherent phase-space rotations of the nanocavity field using a tip nanoprobe, and discuss the tunable role of molecular anharmonicity as a function of pump power. Our work offers microscopic design strategies for quantum state preparation and control with emitter-nanocavity hybrids using infrared quantum optics.
Individual members of an ensemble of identical systems coupled to
a common probe can become entangled with one another, even when they
do not interact directly. We investigate how this type of multipartite entanglement is generated in the context of a system consisting of an ensemble of N two-level atoms resonantly coupled to a single mode of the electromagnetic field. In the case where N=2, the dynamical evolution is studied in terms of the entanglements in the different bipartite divisions of the system, as quantified by the I-tangle. We also propose a generalization of the so-called residual tangle that quantifies the inherent three-body correlations in this tripartite system. This allows us to give a complete characterization of the phenomenon of entanglement sharing in the case of the two-atom Tavis-Cummings model. We also introduce an entanglement monotone which constitutes a lower bound on the I-tangle of an arbitrary bipartite system. This measure is seen to be useful in quantifying the entanglement in various bipartite partitions of the TCM in the case where N > 2, i.e., when there is no known analytic form for the I-tangle.
Stabilizing quantum algorithms against external perturbations and preserving quantum coherence are main challenges in the area of quantum information processing. In this contribution main ideas underlying a new class of recently proposed embedded error-correcting quantum codes are discussed. These detected-jump correcting quantum codes are capable of stabilizing distinguishable qubits against spontaneous decay provided these decay processes originate from couplings to statistically independent reservoirs. Exploiting the classical information about which qubit has been affected by the environment these embedded quantum codes minimize the number of required control measurements and recovery operations as well as redundancy. Their stabilizing properties are exemplified by applying them to Grover's quantum search algorithm.
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